You can uninstall or removes an installed letsencrypt.sh package itself from Ubuntu 17.04 (Zesty Zapus) through the terminal,
$ sudo apt-get remove letsencrypt.sh
If you would like to remove letsencrypt.sh and it's dependent packages which are no longer needed from Ubuntu,
$ sudo apt-get remove --auto-remove letsencrypt.sh
If you use with purge options to letsencrypt.sh package all the configuration and dependent packages will be removed.
$ sudo apt-get purge letsencrypt.sh
If you use purge options along with auto remove, will be removed everything regarding the package, It's really useful when you want to reinstall again.
$ sudo apt-get purge --auto-remove letsencrypt.sh